Multidecadal Changes in Lower Stratospheric Ozone: Variability Vs. Trends

[摘要] As upper stratospheric ozone appears to be recovering as a result of decreasing chlorine loading following the implementation of the Montreal Protocol and its amendments and in agreement with model projections, several recent studies report an apparent decline of ozone concentrations in the lower stratosphere in the last two decades, particularly in the extratropics. Our previous work as well as at least two other studies provide evidence that this decline results from transport changes rather than an intensification of chemical depletion. It remains unclear whether these changes represent long-term internal variability or are a consequence of a climate forcing. Here we perform free-running ensembles of the recent past (1980-2016) using the Goddard Earth Observing System Model (GEOS) at the cubed sphere C180 (approximately half degree) resolution. Two suites of 10-member ensembles are performed, one in which observed sea surface temperature (SSTs) are fully prescribed, and the other in which the linear SST trend over the recent past is removed so as to only retain internal variability. We evaluate the trends in both ozone as well as two idealized tracers with prescribed uniform loss that are used to isolate the role of transport from chemistry and emissions. Probability-distribution-functions of the trends in both ozone and idealized tracers are compared among ensemble members and with observed trends in order to evaluate the likelihood of recent observed declines in lower stratospheric ozone, relative to large internal variability. Moreover, comparisons among simulations with and without imposed SST trends indicate the extent to which dynamically-driven ozone trends reflect forced trends or internal variability in lower stratospheric dynamics.

[发布日期] 2018-12-10

[学科分类] 大气科学

[关键词] STRATOSPHERE;OZONE;EARTH OBSERVING SYSTEM (EOS);CHLORINE;PROBABILITY DISTRIBUTION FUNCTIONS;TEMPERATE REGIONS;TRENDS;ATMOSPHERIC COMPOSITION;SIMULATION