Catalog of NO x emissions from point sources as derived from the divergence of the NO 2 flux for TROPOMI

[摘要] We present version 1.0 of a global catalog of NO x emissions from point sources, derived from TROPOspheric Monitoring Instrument (TROPOMI) measurements of tropospheric NO 2 for 2018–2019. The identification of sources and quantification of emissions are based on the divergence (spatial derivative) of the mean horizontal flux, which is highly sensitive for point sources like power plant exhaust stacks. The catalog lists 451 locations which could be clearly identified as NO x point sources by a fully automated algorithm, while ambiguous cases as well as area sources such as megacities are skipped. A total of 242 of these point sources could be automatically matched to power plants. Other NO x point sources listed in the catalog are metal smelters, cement plants, or industrial areas. The four largest localized NO x emitters are all coal combustion plants in South Africa. About 1 / 4 of all detected point sources are located in the Indian subcontinent and are mostly associated with power plants. The catalog is incomplete, mainly due to persisting gaps in the TROPOMI NO 2 product at some coastlines, inaccurate or complex wind fields in coastal and mountainous regions, and high noise in the divergence maps for high background pollution. The derived emissions are generally too low, lacking a factor of about 2 up to 8 for extreme cases. This strong low bias results from combination of different effects, most of all a strong underestimation of near-surface NO 2 in TROPOMI NO 2 columns. Still, the catalog has high potential for checking and improving emission inventories, as it provides accurate and independent up-to-date information on the location of sources of NO x and thus also CO 2 . The catalog of NO x emissions from point sources is freely available at https://doi.org/10.26050/WDCC/Quant_NOx_TROPOMI ( Beirle et al. ,  2020 ) .

[学科分类] 眼科学