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Comparative studies of negative ion formation in Rydberg atom collisions with attaching and polar targets
[摘要] Low-energy electron transfer in collisions between a Rydberg atom and a target molecule can result in the formation of negative ions. Depending as to the properties of the target molecule the electron may be bound in a localized molecular orbital (valence-bound) or bound by its dipole potential in a diffuse orbital located at the positive end of the dipole (dipole-bound). Here we examine the properties of valence-bound and dipole-bound negative ions created through electron transfer in collision with Rydberg atoms, in particular, their lifetimes, collisional properties and electric-field-induced detachment characteristics. Intercomparison of the various data also leads to new insights into electron attachment to molecules that can support both valence-bound and dipole-bound negative ion states.
[发布日期]  [发布机构] Rice University
[效力级别] physics [学科分类] 
[关键词]  [时效性] 
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