Measurement of Helium-3/Helium-4 Ratios in Soil Gas at the 618-11 Burial Ground.

[摘要] Seventy soil gas-sampling points were installed around the perimeter of the 618-11 Burial Ground, approximately 400 feet downgradient of well 699-13-3A, and in four transects downgradient of the burial ground to a maximum distance of 3,100 feet. Soil gas samples were collected and analyzed for helium-3/helium-4 ratios from these 70 points. Helium-3/helium-4 ratios determined from the soil gas sampling points showed significant enrichments, relative to ambient air helium-3 concentrations. The highest concentrations were located along the northern perimeter of the burial ground. Helium-3/helium-4 ratios (normalized to the abundances in ambient air) ranged from 1.0 to 62 around the burial ground. The helium-3/helium-4 ratios from the 4 transect downgradient of the burial ground ranged from 0.988 to 1.68. The helium-3/helium-4 ratios from around the burial ground suggest there is a vadose zone source of tritium along the north side of the burial ground.

[发布机构] Technical Information Center Oak Ridge Tennessee

[学科分类] 工程和技术（综合）

[关键词] Radionuclide migration;Helium 3;Soils;Underground storage;Sampling